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Advances in Laser Chemistry: Proceedings of the Conference by S. A. Rice (auth.), Professor Dr. Ahmed H. Zewail (eds.)

By S. A. Rice (auth.), Professor Dr. Ahmed H. Zewail (eds.)

The laser as a radiation resource with temporal and spatial coherence has made an important impression within the assorted fields of technological know-how. consequently, new and intriguing learn has been constructing allover the area. Laser spectro­ scopy stocks a wide fraction of this examine, and within the final decade nu­ merous books and monographs were released in this topic. every one of these books and monographs comprise the paintings performed within the physics group. only a few books symbolize the advances made in laser chemistry, a box that's flourishing and whose destiny is certainly very intriguing. It was once felt assembly that desirous about the $64000 questions being requested within the chemistry neighborhood, and on new and attainable instructions in laser chemistry, was once wanted. This three-day convention, held on the California Institute of expertise, Pasadena, California, on March 20-22, 1978, coated 5 very important parts in laser chemistry: Laser-induced chemistry, picosecond strategies and methods, nonlinear optical spectroscopy and dephasing procedures, multiphoton exci­ tation in molecules, and molecular dynamics through molecular beams.

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Additional resources for Advances in Laser Chemistry: Proceedings of the Conference on Advances in Laser Chemistry, California Institute of Technology, Pasadena, USA, March 20–22, 1978

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Child, Molecular Collision Theory, Academic Press, New York (1974). 39. F. H. Mies, J. Chem. 21, 787, 798 (1969). 40. s. A. Rice, I. Mclaughlin and J. Jortner, J. Chem. Phys. 49, 2756 (1968). 41. K. G. Kay and S. A. Rice, J. Chem. Phys. 57, 3041 (1972). 42. E. J. Heller and S. A. Rice, J. Chem. Phys . l, 936 (1974). 43. M. Muthukumar and S, A. Rice submitted to J. Chem. Phys. 44. K. G. Kay, J. Chem. Phys . l, 5205 (1974). 45. w. M. Gelbart, S. A. Rice and K. F. Freed, J. Chem. 2, 4699 (1972). 46.

It is also illuminating to compare the coverage of the surface of section by the apparently stochastic trajectory with the region of Hilbert space wherein the spectrum is very sensitive to the coupling. LEscape _____ _ 20·0 16-0 Sensitivity of the eigenvalues of the Henon-Heiles model Hamiltonian to small changes in coupling. From [30]. I :. 0 • 8·0 4· 0·004 0-008 A2 0·012 0·016 IIEI 2M Comparison of area of surface of section covered by nonperiodic trajectory, and domain of Hi Ibert space where the ei£lenvalues are sensitive to small changes in coupling, From [30].

P ; given this means choosing Pa ,which implies knowledge of the eigenstates of I{ , and this is just,XIhat is not usually available. ISB and classically. Nordholm and Rice considered a two oscillator coupled system for which ..... /C/~SSit:#I=t(f;Z·+A'1-/-) +1. ) -I-f 0:+ AI. 'fz. I "', <. 'c: • Even withcout the cutoff HC1f/srie. A HIJI7YI" m a dCm,) I m ,, )t'7Z. ). )>;. Gc.. g. by Fano's method. stimated from the classical halflife. 48 are: (i) E:~ varies over a wide range even for e"> £c • The range of variation is larger when the osci lIators are nondegenerate; the variation is irregular.

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